2 Photocatalysis: The Principles

F. Gaida; A. G. Griesbeck; M. Vollmer

doi:10.1055/sos-SD-229-00002

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König, B.: 2019 Science of Synthesis, 2018/6: Photocatalysis in Organic Synthesis DOI: 10.1055/sos-SD-229-00002

Photocatalysis in Organic Synthesis

2 Photocatalysis: The Principles

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Buch

Herausgeber: König, B.

Autoren: Akita, M.; Albero, J.; Amador, A. G.; Ashley, M. A.; Brasholz, M.; Corcé, V.; DiRocco, D. A.; Dix, S.; Ehrnsberger, P.; Fensterbank, L.; Gaida, F.; García, H.; Ghosh, I.; Gilmour, R.; Griesbeck, A. G.; Gutiérrez Bonet, Á.; Hepburn, H. B.; Hopkinson, M. N.; Kelly, C. B.; Koike, T.; Laha, R.; Lang, S. B.; Leonori, D.; Lévêque, C.; Li, P.; Lu, L.-Q.; Matsui, J. K.; Melchiorre, P.; Metternich, J. B.; Molander, G. A.; Mudd, R. J.; Ollivier, C.; Pandey, G.; Phelan, J. P.; Reiser, O.; Rey, Y. P.; Rovis, T.; Ruffoni, A.; Scholz, S. O.; Schultz, D. M.; Skubi, K. L.; Speckmeier, E.; Thullen, S. M.; Vollmer, M.; Wang, L.; Wang, M.; Wei, Y.; Xiao, W.-J.; Yoon, T. P.; Zeitler, K.; Zhou, Q.-Q.

Titel: Photocatalysis in Organic Synthesis

Print ISBN: 9783132417021; Online ISBN: 9783132417069; Buch-DOI: 10.1055/b-006-161273

1st edition © 2019. Thieme. All rights reserved.
Georg Thieme Verlag KG, Stuttgart

Fachgebiete: Organische Chemie;Chemische Reaktionen, Katalyse;Organometallchemie;Chemische Labormethoden, Stöchiometrie

Science of Synthesis Reference Libraries

Übergeordnete Publikation

Titel: Science of Synthesis

DOI: 10.1055/b-00000101

Reihenherausgeber: Fürstner, A. (Editor-in-Chief); Carreira, E. M.; Faul, M.; Kobayashi, S.; Koch, G.; Molander, G. A.; Nevado, C.; Trost, B. M.; You, S.-L.

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Abstract

Understanding photocatalysis requires knowledge of the primary and secondary photophysical and photochemical processes: light absorption and emission, radiationless decay, energy and electron transfer, and hydrogen and group transfer. Photocatalysis is largely dictated by energy and spin restrictions that allow fast transfer of energy, electrons, or atoms. The kinetics of photoredox-initiated catalysis can be estimated from the redox properties of the electronic ground states as well as the excitation energies and spin properties of the excited states involved. These principles are demonstrated using three model processes: photochemical decarboxylation, fluorination/fluoroalkylation, and (molecular) oxygen-transfer processes.

Schlüsselwörter

photocatalysis - photochemistry - photolysis - homogeneous catalysis - heterogeneous catalysis - asymmetric catalysis - transition-metal catalysis - ruthenium catalysts - iridium catalysts

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