Mascareñas, J. L. et al.: Science of Synthesis: Abiotic Reactions in Live Environments DOI: 10.1055/sos-SD-242-00020

14 Bioorthogonal Strategies for the Uncaging and Assembly of Drugs

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Book

Editors: Mascareñas, J. L.; Tomás-Gamasa, M.

Authors: Jeong, Y.; Winssinger, N.; Taran, F.; Kohyama, A.; Papot, S.; Porte, K.; Unciti-Broceta, A.; Jin, S.; Adam, C.; Lorente-Macías, Á.; Croke, S.; Thoreau, F.; Geng, J. ; Lin, S. ; Sapkota, N.

Title: Abiotic Reactions in Live Environments

Online ISBN: 9783132458277; Book DOI: 10.1055/b000000918

Subjects: Organic Chemistry;Chemical Reactions, Catalysis;Laboratory Techniques, Stoichiometry;Biochemistry;Pharmaceutical Chemistry, Medizinische Chemie

Science of Synthesis Reference Libraries



Parent publication

Title: Science of Synthesis

DOI: 10.1055/b-00000101

Series Editors: Fürstner, A. (Editor-in-Chief); Carreira, E. M.; Faul, M.; Kobayashi, S.; Koch, G.; Molander, G. A.; Nevado, C.; Trost, B. M.; You, S.-L.

Type: Multivolume Edition

 


Abstract

The bioorthogonal synthesis of drugs offers a unique opportunity for targeting — either molecularly, spatiotemporally or both — the delivery of active compounds directly to the disease site. Problems such as unfavorable pharmacokinetic (PK) profiles and dose-limiting side effects can be mitigated with the careful deployment of the tools of biorthogonal chemistry. In order to access medicinal applications, researchers have developed groundbreaking new chemistries for the caging and uncaging, assembly, and molecular targeting of a wide range of clinically approved drugs. This review presents notable examples of bioorthogonal drug synthesis that have emerged from the two main branches of the bioorthogonal field: organic click chemistries and transition-metal-catalyzed reactions.

 
  • 7 Rubio-Ruiz B, Bray TL, López-Pérez AM, Unciti-Broceta A, Coupling and Decoupling of Diverse Molecular Units in Glycosciences. Witczak ZJ, Bielski R. Springer; Cham, Switzerland 2018: 269
  • 25 Scinto SL, Bilodeau DA, Hincapie R, Lee W, Nguyen SS, Xu M, am Ende CW, Finn MG, Lang K, Lin Q, Pezacki JP, Prescher JA, Robillard MS, Fox JM. Nat. Rev. Methods Primers 2021; 1: 30
  • 26 Rossin R, Versteegen RM, Wu J, Khasanov A, Wessels HJ, Steenbergen EJ, ten Hoeve W, Janssen HM, van Onzen AHAM, Hudson PJ, Robillard MS. Nat. Commun. 2018; 9: 1484
  • 27 Jiménez-Moreno E, Guo Z, Oliveira BL, Albuquerque IS, Kitowski A, Guerreiro A, Boutureira O, Rodrigues T, Jiménez-Osés G, Bernardes GJL. Angew. Chem. Int. Ed. 2017; 56: 243
  • 42 Pérez-López AM, Rubio-Ruiz B, Sebastián V, Hamilton L, Adam C, Bray TL, Irusta S, Brennan PM, Lloyd-Jones GC, Sieger D, Santamaría J, Unciti-Broceta A. Angew. Chem. Int. Ed. 2017; 56: 12548
  • 43 Oliveira BL, Stenton BJ, Unnikrishnan VB, Rebelo de Almeida C, Conde J, Negrão M, Schneider FSS, Cordeiro C, Godinho Ferreira M, Caramori GF, Domingos JB, Fior R, Bernardes GJL. J. Am. Chem. Soc. 2020; 142: 10869
  • 45 Weiss JT, Dawson JC, Macleod KG, Rybski W, Fraser C, Torres-Sánchez C, Patton EE, Bradley M, Carragher NO, Unciti-Broceta A. Nat. Commun. 2014; 5: 3277
  • 51 Dal Forno GM, Latocheski E, Machado AB, Becher J, Dunsmore L, St. John AL, Oliveira BL, Navo CD, Jiménez-Osés G, Fior R, Domingos JB, Bernardes GJL. J. Am. Chem. Soc. 2023; 145: 10790
  • 53 Pérez-López AM, Rubio-Ruiz B, Valero T, Contreras-Montoya R, Álvarez de Cienfuegos L, Sebastián V, Santamaría J, Unciti-Broceta A. J. Med. Chem. 2020; 63: 9650
  • 55 Hoop M, Ribeiro AS, Rösch D, Weinand P, Mendes N, Mushtaq F, Chen X.-Z, Shen Y, Pujante CF, Puigmartí-Luis J, Paredes J, Nelson BJ, Pêgo AP, Pané S. Adv. Funct. Mater. 2018; 28: 1705 920
  • 70 Southwell JW, Herman R, Raines DJ, Clarke JE, Böswald I, Dreher T, Gutenthaler SM, Schubert N, Seefeldt J, Metzler-Nolte N, Thomas GH, Wilson KS, Duhme-Klair A.-K. Chem.–Eur. J. 2023; 29: e202202536
  • 76 Rubio-Ruiz B, Pérez-López AM, Uson L, Ortega-Liebana MC, Valero T, Arruebo M, Hueso JL, Sebastian V, Santamaria J, Unciti-Broceta A. Nano Lett. 2023; 23: 804
  • 88 van de LʼIsle M, Croke S, Valero T, Unciti-Broceta A. Chem.–Eur. J. 2024; e202400611
  • 93 Wang C, Zhang H, Zhang T, Zou X, Wang H, Rosenberger JE, Vannam R, Trout WS, Grimm JB, Lavis LD, Thorpe C, Jia X, Li Z, Fox JM. J. Am. Chem. Soc. 2021; 143: 10793