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CC BY 4.0 · SynOpen 2023; 07(01): 88-101
DOI: 10.1055/a-2035-6733
DOI: 10.1055/a-2035-6733
graphical review
Amide N–C Bond Activation: A Graphical Overview of Acyl and Decarbonylative Coupling
We thank the National Science Foundation (NSF) (CAREER CHE-1650766), the National Institutes of Health (NIH) (R35GM133326), Rutgers University, the Overseas High-Level Talents Fund of Shanghai, and Shanghai University for generous support.
Abstract
This Graphical Review provides an overview of amide bond activation achieved by selective oxidative addition of the N–C(O) acyl bond to transition metals and nucleophilic acyl addition, resulting in acyl and decarbonylative coupling, together with key mechanistic details pertaining to amide bond distortion underlying this reactivity manifold.
Key words
C–N activation - amide bond activation - acyl coupling - decarbonylative coupling - acyl addition - catalysisPublication History
Received: 13 January 2023
Accepted after revision: 14 February 2023
Accepted Manuscript online:
14 February 2023
Article published online:
06 March 2023
© 2023. The Author(s). This is an open access article published by Thieme under the terms of the Creative Commons Attribution License, permitting copying and reproduction so long as the original work is given appropriate credit. Contents may not be used for commercial purposes or adapted, remixed, transformed or built upon. (https://creativecommons.org/licenses/by/4.0/)
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