Synthesis 2017; 49(06): 1307-1314
DOI: 10.1055/s-0036-1588090
paper
© Georg Thieme Verlag Stuttgart · New York

Chiral Primary Amine–Squaramide Catalyzed Highly Enantio­selective Michael Addition of Isobutyraldehyde to Nitroolefins

Zhi-Wei Ma*
a   Department of Fundamental Courses, Henan University of Animal Husbandry and Economy, No. 2 Yingcai Street, Huiji District, Zhengzhou 450044, Henan, P. R. of China   Email: mazhiwei1986@126.com
,
Xiao-Feng Liu
b   College of Chemistry and Molecular Engineering, Zhengzhou University, No. 100 Science Avenue, High-Tech Zone, Zhengzhou 450001, Henan, P. R. of China   Email: jctao@zzu.edu.cn
,
Bin Sun
b   College of Chemistry and Molecular Engineering, Zhengzhou University, No. 100 Science Avenue, High-Tech Zone, Zhengzhou 450001, Henan, P. R. of China   Email: jctao@zzu.edu.cn
,
Xian-Hui Huang
b   College of Chemistry and Molecular Engineering, Zhengzhou University, No. 100 Science Avenue, High-Tech Zone, Zhengzhou 450001, Henan, P. R. of China   Email: jctao@zzu.edu.cn
,
Jing-Chao Tao*
b   College of Chemistry and Molecular Engineering, Zhengzhou University, No. 100 Science Avenue, High-Tech Zone, Zhengzhou 450001, Henan, P. R. of China   Email: jctao@zzu.edu.cn
› Author Affiliations
Further Information

Publication History

Received: 31 August 2016

Accepted after revision: 14 October 2016

Publication Date:
22 November 2016 (online)


Abstract

Chiral primary amine–squaramides have not been extensively studied to date in the field of organocatalysis. In this paper, novel chiral squaramides derived from natural product stevioside were developed. Both enantiomers of a series of γ-nitroaldehydes were generated by using these squaramide catalysts for the Michael addition reaction of isobutyraldehyde to nitroolefins. This asymmetric reaction proceeded well to afford the desired products in high yields (up to 98%) with high to excellent enantioselectivities (up to 99% ee).

Supporting Information

 
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