Synthesis 2019; 51(12): 2579-2583
DOI: 10.1055/s-0037-1610703
paper
© Georg Thieme Verlag Stuttgart · New York

Reactions of t-Boc-Protected Amines with Difluorocarbene

Andrii Gerasov
a   Life Chemicals Inc., Murmanska st. 5, Kyiv, 02660, Ukraine   Email: A.Shivanyuk@lifechemicals.com
,
Alexander Shivanyuk*
a   Life Chemicals Inc., Murmanska st. 5, Kyiv, 02660, Ukraine   Email: A.Shivanyuk@lifechemicals.com
b   The Institute of High Technologies, Taras Shevchenko National University of Kyiv, 4 Glushkov st.5, Kyiv, 03187, Ukraine
,
Volodymyr Fetyukhin
a   Life Chemicals Inc., Murmanska st. 5, Kyiv, 02660, Ukraine   Email: A.Shivanyuk@lifechemicals.com
,
Oleg Lukin
a   Life Chemicals Inc., Murmanska st. 5, Kyiv, 02660, Ukraine   Email: A.Shivanyuk@lifechemicals.com
› Author Affiliations
Further Information

Publication History

Received: 16 January 2019

Accepted after revision: 11 March 2019

Publication Date:
06 May 2019 (online)


Abstract

The reactions of t-Boc-protected secondary and primary amines with difluorocarbene generated from trimethylsilyl (fluorosulfonyl)difluoroacetate [Me3SiOC(O)CF2SO2F] (TFDA) in toluene at 110 °C results in the replacement of t-Bu by difluoromethyl in the t-Boc group. This reaction can be carried out in the presence of CH2Br and COOMe moieties in the structure of the protected amine. In the example of a t-Boc-protected amine containing a C=C double bond, replacement of the t-Bu group and/or cyclodifluoropropanation takes place. Difluoromethyl esters are shown to react with primary and secondary amines yielding the corresponding ureas.

Supporting Information

 
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