Cu-Catalyzed Tandem Friedel-Crafts/Henry Reaction

doi:10.1055/s-2008-1078663

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Synfacts 2008(9): 0953-0953
DOI: 10.1055/s-2008-1078663

Metal-Catalyzed Asymmetric Synthesis and Stereoselective Reactions

Cu-Catalyzed Tandem Friedel-Crafts/Henry Reaction

Contributor(s): Hisashi Yamamoto, Marina Naodovic
T. Arai*, N. Yokoyama
Chiba University, Japan

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Publikationsdatum:
22. August 2008 (online)

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Significance

This report describes one of the first successful tandem Friedel-Crafts/Henry (FCH) reactions that provide acyclic chiral products. The most significant point of this account is the predominant formation of only three diastereomers of the three-component reaction products (3) that bear three contiguous stereocenters.